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The separation of xylene isomers still remains an industrially challenging task. Here, porous purine-based metal–organic frameworks (MOFs) have been synthesized and studied for their potential in xylene separations. In particular, Zn(purine)I showed excellent para -xylene/ ortho -xylene separation capability with a diffusion selectivity of 6 and high equilibrium adsorption selectivity as indicated by coadsorption experiments. This high selectivity is attributed to the shape and size of the channel aperture within the rigid framework of Zn(purine)I.more » « less
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Zhou, Xiuquan ; Malliakas, Christos D. ; Yakovenko, Andrey A. ; Wilfong, Brandon ; Wang, Suyin G. ; Chen, Yu-Sheng ; Yu, Lei ; Wen, Jianguo ; Balasubramanian, Mahalingam ; Wang, Hsien-Hau ; et al ( , Nature Synthesis)